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Accuracy and precision of the RABBIT technique

One of the most ubiquitous techniques within attosecond science is the so-called reconstruction of attosecond beating by interference of two-photon transitions (RABBIT). Originally proposed for the characterization of attosecond pulses, it has been successfully applied to the accurate determination of time delays in photoemission. Here, we examine in detail, using numerical simulations, the effect

Inorganic Ions Assisted Anisotropic Growth of CsPbCl3 Nanowires with Surface Passivation Effect

All-inorganic halide perovskite nanowires (NWs) exhibit improved thermal and hydrolysis stability and could thus play a vital role in nanoscale optoelectronics. Among them, blue-light-based devices are extremely limited because of the lack of a facile method to obtain high-purity CsPbCl3 NWs. Herein, we report a direct and facile method for the synthesis of CsPbCl3 NWs assisted by inorganic ions t

Surface Engineering of Quantum Dots for Remarkably High Detectivity Photodetectors.

Ternary alloyed CdSexTe1–x colloidal QDs trap-passivated by iodide-based ligands (TBAI) are developed as building blocks for UV–NIR photodetectors. Both the few surface traps and high loading of QDs are obtained by in situ ligand exchange with TBAI. The device is sensitive to a broad wavelength range covering the UV–NIR region (300–850 nm), showing an excellent photoresponsivity of 53 mA/W, a fast

Rotating Binary Bose-Einstein Condensates and Vortex Clusters in Quantum Droplets

Quantum droplets may form out of a gaseous Bose-Einstein condensate, stabilized by quantum fluctuations beyond mean field. Determining the ground state of a rotating binary condensate, we show that multiple singly quantized vortices may form in these droplets at moderate angular momenta in two dimensions. Droplets carrying these precursors of an Abrikosov lattice remain self-bound for certain time

Charge-photon transport statistics and short-time correlations in a single quantum dot-resonator system with an arbitrarily large coupling parameter

Electrical quantum conductors coupled to microwave resonators have in the last decade emerged as a versatile test bed for controllable light-matter interaction on the nanometer scale. Recent experimental progress with high-impedance resonators has resulted in conductor-resonator systems with a large, dimensionless coupling parameter λ 0.1, well beyond the small-coupling regime, λ1 Motivated by thi

Voltage-manipulating graphene-mediated surface-enhanced Raman scattering (G-SERS) : principle and applications

The voltage-controlled graphene-mediated surface-enhanced Raman scattering (G-SERS) spectroscopy is experimentally developing spectral technology, and which is prosperously applied in the fields of ultra-sensitive spectral analysis, sensor and catalysis. In this review, we introduce the physical principle, fabrication method, and recent applications of voltage-controlled G-SERS. We firstly introdu

X-ray Spectrometer

An x-ray spectrometer includes: an x-ray plasma source that produces first x-rays; an x-ray optic in optical communication with the x-ray plasma source and that: receives the first x-rays from the x-ray plasma source; focuses the first x-rays to produce second x-rays; and communicates the second x-rays to a sample that produces product x-rays in response to receipt of the second x-rays and second

Association Between Vitamin D, Frailty, and Progression of Frailty in Community-Dwelling Older Women

CONTEXT: Vitamin D (25OHD) is involved in many physiological functions that decline with age, contributing to frailty and increased risk for negative health outcomes. Whether 25OHD is a long-term risk marker for frailty over a longer time and whether it is consistent with advancing age is unclear. OBJECTIVE: To investigate the association between 25OHD and frailty in older women followed for 10 ye

Photo-Oxidation Reveals H-Aggregates Hidden in Spin-Cast-Conjugated Polymer Films as Observed by Two-Dimensional Polarization Imaging

Spin-cast intermolecular interactions in conjugated polymer films lead to the formation of excited states delocalized over a few oriented and tightly packed conjugated segments. The optoelectronic properties of conjugated polymers are strongly dependent on the presence of such oriented domains at a nanoscale level. We observe oriented domains as large as several micrometers in size spontaneously f

Thermodynamic uncertainty relations including measurement and feedback

Thermodynamic uncertainty relations quantify how the signal-to-noise ratio of a given observable is constrained by dissipation. Fluctuation relations generalize the second law of thermodynamics to stochastic processes. We show that any fluctuation relation directly implies a thermodynamic uncertainty relation, considerably increasing their range of applicability. In particular, we extend thermodyn

Compact single-shot D-scan setup for the characterization of few-cycle laser pulses

Ultrashort laser pulses have become an indispensable tool in physics, chemistry and engineering. Their numerous applications call for accurate and robust characterization techniques able to reliably retrieve the pulse's intensity profile. Different methods, such as FROG [1] or SPIDER [2] and their variants, have been developed in past decades and are now common in many laboratories. More novel app

An introduction to attosecond pulses and attosecond physics

The interaction of atoms with intense laser radiation leads to the generation of high-order harmonics of the laser field. In the time domain, this corresponds to a train of pulses in the extreme ultraviolet range and with attosecond duration. This tutorial will introduce the physics of high-order harmonic generation and attosecond pulses.

Soliton self-compression and spectral broadening of 1 μm femtosecond pulses in single-domain KTiOPO4

Efficient, diode-pumped high energy femtosecond laser systems around 1 μm based on Yb-gain media are readily commercially available. However, owing to the gain bandwidth limitations, the pulses generated in such lasers are substantially longer than the ones generated in Ti:Sapphire systems. A simple, energy-scalable pulse self-compression scheme for the pulses around 1 μm thus would be of great in

Femtosecond streaking and control of electrons from a plasmonic nanofocusing taper by photoemitted charges in a nanoantenna

Manipulation of electrons by light forms the basis for future optoelectronic devices targeting switching speeds close to optical frequencies. Specifically, nanolocalized optical and plasmonic fields play a key role as they reduce the interaction region down to few nanometers and thus the time electrons require to traverse the fields. In this context, the precise knowledge of the localized fields i

Precision public health: mapping socioeconomic disparities in opioid dispensations at Swedish pharmacies by Multilevel Analysis of Individual Heterogeneity and Discriminatory Accuracy (MAIHDA)

BackgroundIn light of the opioid epidemic in the United States, there is growing concern about the use of opioids in Sweden as it may lead to misuse and overuse and, in turn, severe public health problems. However, little is known about the distribution of opioid use across different demographic and socioeconomic dimensions in the Swedish general population. Therefore, we applied an intersectional

Understanding the Lipid and Protein Corona Formation on Different Sized Polymeric Nanoparticles

When in contact with biological fluids, nanoparticles dynamically absorb biomolecules like proteins and lipids onto their surface, forming a “corona”. This biocorona is a dynamic and complex structure that determines how host cells respond to nanoparticles. Despite the common use of mouse models in pre-clinical and toxicological experiments, the impact of corona formed in mouse serum on the biophy

Large lattice distortions and size-dependent bandgap modulation in epitaxial halide perovskite nanowires

Metal-halide perovskites have been shown to be remarkable and promising optoelectronic materials. However, despite ongoing research from multiple perspectives, some fundamental questions regarding their optoelectronic properties remain controversial. One reason is the high-variance of data collected from, often unstable, polycrystalline thin films. Here we use ordered arrays of stable, single-crys

Breakup dynamics of gas-liquid interface during Taylor bubble formation in a microchannel flow-focusing device

This work aims to investigate the breakup dynamics of the gas-liquid interface during bubble formation in a microchannel flow-focusing device. An interface tracking method is developed to capture the profiles of the gaseous thread evolution. The results show that the pinch-off period can be further divided into a liquid squeezing stage and a free pinch-off stage in both the radial and axial direct